Investigation of Second- and Third-Harmonic Generation in Few-Layer Gallium Selenide by Multiphoton Microscopy

نویسندگان

  • Lasse Karvonen
  • Antti Säynätjoki
  • Soroush Mehravar
  • Raul D. Rodriguez
  • Susanne Hartmann
  • Dietrich R. T. Zahn
  • Seppo Honkanen
  • Robert A. Norwood
  • N. Peyghambarian
  • Khanh Kieu
  • Harri Lipsanen
  • Juha Riikonen
چکیده

Gallium selenide (GaSe) is a layered semiconductor and a well-known nonlinear optical crystal. The discovery of graphene has created a new vast research field focusing on two-dimensional materials. We report on the nonlinear optical properties of few-layer GaSe using multiphoton microscopy. Both second- and third-harmonic generation from few-layer GaSe flakes were observed. Unexpectedly, even the peak at the wavelength of 390 nm, corresponding to the fourth-harmonic generation or the sum frequency generation from third-harmonic generation and pump light, was detected during the spectral measurements in thin GaSe flakes.

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عنوان ژورنال:

دوره 5  شماره 

صفحات  -

تاریخ انتشار 2015